Not much unless u spray,supercharged/turbo it.There are some mods depending on your emissions regulations.If you really want to keep the six I would do a blow thru turbo setup with some sort of bonnet/enclosure or put small block chevy in it.
As for mods for the N/A 231
4.1 4barrel intake,or edelbrock perfomer buick kit includes cam,intake,CARB
Change the gears most g-body 231 usually have 2.41-2.73 change to 3.23 or 3.42.