Big can of worms with this one.....
Good thread though.
I agree with all that has been said. Higher CR will help spool up slightly. It's not the cure all. N2O is the quickest method for spooling any turbo, that is true, but it brings more tuning issues into the picture. Namely, if your chip (assuming that you're using a stock ECM) is not burned for N2O use, it will have too much timing and could cause some dangerous lean conditions which could pop a head gasket or two. If you intend to run N2O, you must have a proper tune to compensate for the sudden lean spike that occurs.
The only thing I can say, that will help explain how the CR helps spoolup is,
higher CR creates more exhaust velocity and higher EGT temps at lower rpms.
These are the main two factors that contribute the most too help spool up a large turbine wheel that are engine specific.
And the current 70 series turbos that are out there, have large turbine wheels, as compaired to what 95% of the Turbo Buick world normally runs on a street car. The only other factor that can greatly contribute to quicker spool, other than N2O, would be reducing the engines accessory drive rotating mass. IE: Billet aluminum crank pulley, water pump pulley (the extreme being eliminating the belt driven water pump and going with an electric water pump) PS pump pulley, alternator pulley, light weight 9" or 9.5" torque converter vs the stock 12" D5 converter. (easily worth 30#s right there) aluminum driveshaft, and light weight wheels.
Given, the wheels are slightly different than accessory drive and drivetrain rotating mass, but it has been said that removing 1# of rotating mass is the same as removing 7#s of static weight. In the past, I have seen gains from doing all of these items above on street cars. Especially the torque converter, light weight wheels and billet crank pulley. Those 3 items significantly helped with helping the motor rev quickly. With the tuning features that a Turbo Tweak chip have (namely allowing you to pull fuel out on spool up) can help your spool up even more.
Me personally, if you know you will never see any better gas than 93 octane, and will be street driving 95% of the time, I would suggest staying with 8.5:1 CR. If you plan on running straight 100-103 octane unleaded all the time, or alky injection under boost, then by all means, go with 9.0:1. Just remember, that you will limit yourself to the maximum allowable boost that you can physically run before you start popping head gaskets on our 4 bolt per cylinder style heads. I've had friends pop head gaskets at 30psi on C16 on a motor that had 9.0:1 CR, given the tune could have been bad, or detonation could have loosened up the gaskets in a previous pass, but it's just some things to consider. Also, you shouldn't have to run 30-35psi of boost to reach your goals to begin with. If you are having to run that much boost, you definitely have the wrong turbo on your combo.
The ideal selection with our little 231-235 motors, would be to have a turbo that only has to run 24-26psi to reach your goals and spool up as fast as a stocker. If your goals are mid to high 9's on a 235CI, you would need to run a larger than 70mm size comp wheel, as very, very few people with full weight (3650 lb+) Buicks, have accomplished this goal without the help of N2O. Sure, spraying a 235CI production motor with a good cam and maxed out aluminum heads would easily run 9's, but, just how long will the head gaskets stay in one piece?????? It sure doesn't take much to pop a head gasket, especially with the unequalized distribution of air to each cylinder factor working against us. Then you throw N2O into the mix and you have no way of controlling how much nitrous each cylinder takes, unless you plumb up a direct port N2O kit.
Sorry it's so long winded, just some of my thoughts.
Patrick